MeloDroid is a Windows program that acts as a server for the remote, and allows you to USB sync your Android phone with iTunes (including playlists). It has some useful features in addition to this, such as the ability to disable iTunes services that you don't use (like Bonjour and iTunesHelper) and display Now Playing song notifications. It even gives you the option to shut down iTunes automatically when you're not using it, and starts it back up when you are.
What's new in this version:
Version 5.1.3 has fixed play next problems, and QuickSync bugs.